我组赵雅洁在Applied catalysis B: Environment上发表论文

题目：

Carbon nitride assisted 2D conductive metal-organic frameworks composite photocatalyst for efficient visible light-driven H₂O₂ production

作者：

Yajie Zhao ^a, Yan Liu ^a, Zhenzhen Wang ^a, Yurong Ma ^a, Yunjie Zhou ^a, Xiaofei Shi ^a, Qingyao Wu ^a, Xiao Wang ^a, Mingwang Shao ^a, Hui Huang ^a,**, Yang Liu ^a,**, Zhenhui Kang ^a,b,*

单位：

^a Institute of Functional Nano and Soft Materials Laboratory (FUNSOM), Jiangsu Key Laboratory for Carbon-Based Functional Materials & Devices, Soochow University, Suzhou 215123, PR China

^b Macao Institute of Materials Science and Engineering, Macau University of Science and Technology, Taipa 999078, Macau SAR, PR China

摘要：

To overcome the problems existing in the current H₂O₂ production process, photo-assisted H₂O₂ production by oxygen reduction was studied extensively. Ni-CAT, a 2D conductive hexagonal MOF, shows great potential for photocatalytic H₂O₂ production. However, it has not been developed and utilized as the main photocatalyst. Here, we constructed a C3N4 assisted Ni-CAT composite catalyst, which can achieve the H₂O₂ production by 2e^- oxygen reduction reaction under visible light. During the reaction process, Ni-CAT is the main active component for oxygen reduction reaction, and the role of C₃N₄ is to assist Ni-CAT by providing electrons to inhibit its carrier recombination. This work opens up the application of 2D conductive MOFs in photocatalytic H₂O₂ production and provides a theoretical model for the design of MOFs-based photocatalyst.

影响因子：

16.683

分区情况：

1区

链接：  

https://www.sciencedirect.com/science/article/pii/S0926337321001612?via%3Dihub