题目：

High-Performance, Ultra-Flexible and Transparent Embedded Metallic Mesh Electrodes by Selective Electrodeposition for All-Solid-State Supercapacitor Applications

作者：

Yan-Hua Liu,^a Jian-Long Xu,^*b Su Shen,^*a Xin-Lei Cai,^b Lin-Sen Chen^a and Sui-Dong Wang^*b

单位：

^aCollege of Physics, Optoelectronics and Energy, Key Lab of Advanced Optical Manufacturing Technologies of Jiangsu Province, Key Lab of Modern Optical Technologies of Education Ministry of China, Soochow University, Suzhou, Jiangsu 215006, PR China.

^bInstitute of Functional Nano & Soft Materials (FUNSOM), Jiangsu Key Laboratory for Carbon-Based Functional Materials & Devices, Soochow University, Suzhou, Jiangsu 215123, PR China. 

摘要：

A novel approach to fabricate large-scale embedded metallic mesh transparent conductive electrodes (TCEs) on flexible substrates via a low-cost and facile selective electrodeposition process combined with inverted film-processing methods is proposed for the first time. The optimized embedded Ni mesh TCEs on polyethylene terephthalate (PET) exhibit excellent optoelectronic properties (R_s ~ 0.2 Ω sp^-1 & T~84%), high figure of merit (FOM~1.0×10^-4) and mechanical durability properties, which arise from the embedded inverted T-type shape of the electrodeposited Ni mesh. The resultant embedded Ni mesh/ polymer poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS) hybrid electrodes are utilized both as current collectors and active electrode materials for all-solid-state flexible transparent supercapacitors, which show high transparency, superior electrochemical performances, excellent mechanical flexibility and high capacitance retention. Even after 1000 cycles of repetitive bending with a radius of 2 mm, the capacitance exhibited a decrease within only 5.2%. The high performance can be attributed to the excellent optoelectronic properties of embedded Ni mesh electrodes in combination with superior electrochemical properties of PEDOT:PSS. This provides a simple, cheap and controllable method for fabricating high-performance flexible TCEs and thus constructing flexible and transparent energy conversion and storage devices and systems.

影响因子：

8.8669

分区情况：

一区

链接：

http://pubs.rsc.org/en/Content/ArticleLanding/2017/TA/C7TA01947E#!divAbstract

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