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康振辉教授课题组在Inorganic Chemistry Frontiers上发表论文
发布时间:2017-10-01 点击:1181

题目:

One-step Synthesis of CoO/g-C3N4 Composites by Thermal Decomposition for Overall Water Splitting without Sacrificial Reagents


作者:

Mumei Han, Huibo Wang, Siqi Zhao, Lulu Hu, Hui Huang* and Yang Liu*


单位:

Jiangsu Key Laboratory for Carbon-based Functional Materials and Devices, Institute of Functional Nano and Soft Materials (FUNSOM), Soochow University, Suzhou, 215123, China.


摘要:

Using photocatalysts to split water into hydrogen and oxygen is a promising way to produce renewable energy. The efficient and stable photaocatalysts are desired for overall water splitting under visible light. We demonstrate the Cobalt (II) oxide (CoO)/graphitic carbon nitride (CoO/g-C3N4) composites synthesized by one-step thermal decomposition method exhibit enhanced photocatalytic efficiency for overall water splitting without sacrificial reagents. The 10%CoO/g-C3N4 exhibits optimal photocatalytic performance, where H2 and O2 evolution rates are respectively 0.46 μmol/h and 0.21μmol/h under visible light irradiation without any sacrificial reagents. It is worth mentioning that the H2 and O2 production almost approach the stoichiometric ratio 2:1. The enhanced photocatalytic activity of CoO/g-C3N4 may be ascribed to the efficient charge separation and fast decomposition of H2O2 by CoO.


影响因子:

4.036


分区情况:

二区


链接:

http://pubs.rsc.org/en/content/articlepdf/2017/QI/C7QI00380C




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